Hybrid organic-inorganic solar cells : Case of the all thin film PMeT(Y)/CdS(X) junctions
Identifieur interne : 013053 ( Main/Repository ); précédent : 013052; suivant : 013054Hybrid organic-inorganic solar cells : Case of the all thin film PMeT(Y)/CdS(X) junctions
Auteurs : RBID : Pascal:00-0350397Descripteurs français
- Pascal (Inist)
- Cellule solaire, Conversion photovoltaïque, Dispositif couche mince, Fabrication, Dopage, Dépôt projection, Dépôt électrolytique, Propriété photoélectronique, Courant court circuit, Tension circuit ouvert, Semiconducteur, Polymère conducteur, Thiophène dérivé polymère, Cadmium sulfure, CdS, Cd S, Thiophène(3-méthyl) polymère.
- Wicri :
- concept : Dopage.
English descriptors
- KwdEn :
Abstract
Hybrid organic-inorganic all thin film photovoltaic junctions PMeT(Y)/CdS(X) were investigated, where PMeT(Y) is the conducting polymer poly(3-methylthiophene) doped with various anions Y = CF3SO-3, ClO-4, BF-4, PF-6, and CdS(X) cadmium sulfide doped with various elements X = Cu, Ni, Al, As and Sb. CdS(X) films were spray deposited on conducting and transparent indium-tin oxide (ITO) glass, and PMeT(Y) films were electrodeposited onto the CdS(X) film to form the junction. The electrochemical investigation of the mechanism of electrodeposition and growth of the PMeT(Y) films by means of chronoamperometry, and of the charge transfer behavior of the PMeT(Y)/CdS(X) junctions by means of cyclic voltammetry revealed a strong effect of the nature of Y and X. The same strong effect of Y was also found with PMeT(Y)/ITO junctions, and may have some generality. It was showed that the best quality of contact between the organic and inorganic phases, from an electrochemical viewpoint and in solution, was obtained with the PMeT(PF-6)/CdS(Sb) junction, pointing towards a similarly better photovoltaic performance in solid state. This was indeed the case, and it was found that higher short-circuit current, open-circuit photovoltage and energy conversion efficiency, approaching 4%, could be obtained with this junction.
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<record><TEI><teiHeader><fileDesc><titleStmt><title xml:lang="en" level="a">Hybrid organic-inorganic solar cells : Case of the all thin film PMeT(Y)/CdS(X) junctions</title><author><name sortKey="Nguyen Cong, H" uniqKey="Nguyen Cong H">H. Nguyen Cong</name><affiliation wicri:level="4"><inist:fA14 i1="01"><s1>Laboratoire d'Electrochimie et de Chimie Physique du Corps Solide, UMR ULP/CNRS 7512, Faculté de Chimie, Université Louis Pasteur, 1-4, rue Blaise Pascal</s1><s2>67000 Strasbourg</s2><s3>FRA</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ></inist:fA14><country>France</country><placeName><region type="region" nuts="2">Alsace</region><settlement type="city">Strasbourg</settlement></placeName><orgName type="university">Université Strasbourg 1</orgName></affiliation></author><author><name sortKey="Dieng, M" uniqKey="Dieng M">M. Dieng</name><affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Laboratoire des Semiconducteurs et d'Energie Solaire, Département de Physique, Faculté des Sciences et Techniques, Université Cheikh Anta Diop</s1><s2>Dakar-Fann</s2><s3>SEN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ></inist:fA14><country>Sénégal</country><wicri:noRegion>Dakar-Fann</wicri:noRegion></affiliation></author><author><name sortKey="Sene, C" uniqKey="Sene C">C. Sene</name><affiliation wicri:level="1"><inist:fA14 i1="02"><s1>Laboratoire des Semiconducteurs et d'Energie Solaire, Département de Physique, Faculté des Sciences et Techniques, Université Cheikh Anta Diop</s1><s2>Dakar-Fann</s2><s3>SEN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ></inist:fA14><country>Sénégal</country><wicri:noRegion>Dakar-Fann</wicri:noRegion></affiliation></author><author><name sortKey="Chartier, P" uniqKey="Chartier P">P. Chartier</name><affiliation wicri:level="4"><inist:fA14 i1="01"><s1>Laboratoire d'Electrochimie et de Chimie Physique du Corps Solide, UMR ULP/CNRS 7512, Faculté de Chimie, Université Louis Pasteur, 1-4, rue Blaise Pascal</s1><s2>67000 Strasbourg</s2><s3>FRA</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ></inist:fA14><country>France</country><placeName><region type="region" nuts="2">Alsace</region><settlement type="city">Strasbourg</settlement></placeName><orgName type="university">Université Strasbourg 1</orgName></affiliation></author></titleStmt><publicationStmt><idno type="inist">00-0350397</idno><date when="2000">2000</date><idno type="stanalyst">PASCAL 00-0350397 INIST</idno><idno type="RBID">Pascal:00-0350397</idno><idno type="wicri:Area/Main/Corpus">012A19</idno><idno type="wicri:Area/Main/Repository">013053</idno></publicationStmt><seriesStmt><idno type="ISSN">0927-0248</idno><title level="j" type="abbreviated">Sol. energy mater. sol. cells</title><title level="j" type="main">Solar energy materials and solar cells</title></seriesStmt></fileDesc><profileDesc><textClass><keywords scheme="KwdEn" xml:lang="en"><term>Cadmium sulfide</term><term>Conducting polymers</term><term>Doping</term><term>Electrodeposition</term><term>Manufacturing</term><term>Open circuit voltage</term><term>Photoelectronic properties</term><term>Photovoltaic conversion</term><term>Semiconductor materials</term><term>Short circuit currents</term><term>Solar cell</term><term>Spray coating</term><term>Thin film device</term><term>Thiophene derivative polymer</term></keywords><keywords scheme="Pascal" xml:lang="fr"><term>Cellule solaire</term><term>Conversion photovoltaïque</term><term>Dispositif couche mince</term><term>Fabrication</term><term>Dopage</term><term>Dépôt projection</term><term>Dépôt électrolytique</term><term>Propriété photoélectronique</term><term>Courant court circuit</term><term>Tension circuit ouvert</term><term>Semiconducteur</term><term>Polymère conducteur</term><term>Thiophène dérivé polymère</term><term>Cadmium sulfure</term><term>CdS</term><term>Cd S</term><term>Thiophène(3-méthyl) polymère</term></keywords><keywords scheme="Wicri" type="concept" xml:lang="fr"><term>Dopage</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Hybrid organic-inorganic all thin film photovoltaic junctions PMeT(Y)/CdS(X) were investigated, where PMeT(Y) is the conducting polymer poly(3-methylthiophene) doped with various anions Y = CF<sub>3</sub>SO<sup>-</sup><sub>3</sub>, ClO<sup>-</sup><sub>4</sub>, BF<sup>-</sup><sub>4</sub>, PF<sup>-</sup><sub>6</sub>, and CdS(X) cadmium sulfide doped with various elements X = Cu, Ni, Al, As and Sb. CdS(X) films were spray deposited on conducting and transparent indium-tin oxide (ITO) glass, and PMeT(Y) films were electrodeposited onto the CdS(X) film to form the junction. The electrochemical investigation of the mechanism of electrodeposition and growth of the PMeT(Y) films by means of chronoamperometry, and of the charge transfer behavior of the PMeT(Y)/CdS(X) junctions by means of cyclic voltammetry revealed a strong effect of the nature of Y and X. The same strong effect of Y was also found with PMeT(Y)/ITO junctions, and may have some generality. It was showed that the best quality of contact between the organic and inorganic phases, from an electrochemical viewpoint and in solution, was obtained with the PMeT(PF<sup>-</sup><sub>6</sub>)/CdS(Sb) junction, pointing towards a similarly better photovoltaic performance in solid state. This was indeed the case, and it was found that higher short-circuit current, open-circuit photovoltage and energy conversion efficiency, approaching 4%, could be obtained with this junction.</div></front></TEI><inist><standard h6="B"><pA><fA01 i1="01" i2="1"><s0>0927-0248</s0></fA01><fA03 i2="1"><s0>Sol. energy mater. sol. cells</s0></fA03><fA05><s2>63</s2></fA05><fA06><s2>1</s2></fA06><fA08 i1="01" i2="1" l="ENG"><s1>Hybrid organic-inorganic solar cells : Case of the all thin film PMeT(Y)/CdS(X) junctions</s1></fA08><fA11 i1="01" i2="1"><s1>NGUYEN CONG (H.)</s1></fA11><fA11 i1="02" i2="1"><s1>DIENG (M.)</s1></fA11><fA11 i1="03" i2="1"><s1>SENE (C.)</s1></fA11><fA11 i1="04" i2="1"><s1>CHARTIER (P.)</s1></fA11><fA14 i1="01"><s1>Laboratoire d'Electrochimie et de Chimie Physique du Corps Solide, UMR ULP/CNRS 7512, Faculté de Chimie, Université Louis Pasteur, 1-4, rue Blaise Pascal</s1><s2>67000 Strasbourg</s2><s3>FRA</s3><sZ>1 aut.</sZ><sZ>4 aut.</sZ></fA14><fA14 i1="02"><s1>Laboratoire des Semiconducteurs et d'Energie Solaire, Département de Physique, Faculté des Sciences et Techniques, Université Cheikh Anta Diop</s1><s2>Dakar-Fann</s2><s3>SEN</s3><sZ>2 aut.</sZ><sZ>3 aut.</sZ></fA14><fA20><s1>23-35</s1></fA20><fA21><s1>2000</s1></fA21><fA23 i1="01"><s0>ENG</s0></fA23><fA43 i1="01"><s1>INIST</s1><s2>18016</s2><s5>354000088993210030</s5></fA43><fA44><s0>0000</s0><s1>© 2000 INIST-CNRS. All rights reserved.</s1></fA44><fA45><s0>13 ref.</s0></fA45><fA47 i1="01" i2="1"><s0>00-0350397</s0></fA47><fA60><s1>P</s1><s2>C</s2></fA60><fA61><s0>A</s0></fA61><fA64 i1="01" i2="1"><s0>Solar energy materials and solar cells</s0></fA64><fA66 i1="01"><s0>NLD</s0></fA66><fC01 i1="01" l="ENG"><s0>Hybrid organic-inorganic all thin film photovoltaic junctions PMeT(Y)/CdS(X) were investigated, where PMeT(Y) is the conducting polymer poly(3-methylthiophene) doped with various anions Y = CF<sub>3</sub>SO<sup>-</sup><sub>3</sub>, ClO<sup>-</sup><sub>4</sub>, BF<sup>-</sup><sub>4</sub>, PF<sup>-</sup><sub>6</sub>, and CdS(X) cadmium sulfide doped with various elements X = Cu, Ni, Al, As and Sb. CdS(X) films were spray deposited on conducting and transparent indium-tin oxide (ITO) glass, and PMeT(Y) films were electrodeposited onto the CdS(X) film to form the junction. The electrochemical investigation of the mechanism of electrodeposition and growth of the PMeT(Y) films by means of chronoamperometry, and of the charge transfer behavior of the PMeT(Y)/CdS(X) junctions by means of cyclic voltammetry revealed a strong effect of the nature of Y and X. The same strong effect of Y was also found with PMeT(Y)/ITO junctions, and may have some generality. It was showed that the best quality of contact between the organic and inorganic phases, from an electrochemical viewpoint and in solution, was obtained with the PMeT(PF<sup>-</sup><sub>6</sub>)/CdS(Sb) junction, pointing towards a similarly better photovoltaic performance in solid state. 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